Efrem Zimbalist Jr.

Following the war, Zimbalist returned to New York and made his Broadway acting debut in The Rugged Path,[10][11] starring Spencer Tracy. This led to a stage career as both actor and producer. His producing successes included bringing three Gian Carlo Menotti operas to Broadway, one of which, The Consul,[12] won the Pulitzer Prize for Music in 1950.

In 1954–1955, he co-starred in his first television series, Concerning Miss Marlowe.[11]

Andra Martin and Zimbalist in 77 Sunset Strip, 1960

Zimbalist in 77 Sunset Strip, 1963

In 1956, Zimbalist was put under contract by Warner Bros. and moved to Hollywood.[13] Zimbalist's first recurring role in a Warner Bros. Television series was as roguish gambler "Dandy Jim Buckley" on Maverick, opposite James Garner in 1957, and making five appearances as the character. In 1958, Zimbalist played the co-lead Stuart "Stu" Bailey in 77 Sunset Strip, a popular detective series running until 1964.

During this period, he made several concurrent appearances in other Warner Bros. television shows, such as Hawaiian Eye, The Alaskans, and Bronco. He also starred as the lead in several feature films for Warners, such as Bombers B-52, The Deep Six, A Fever in the Blood and The Chapman Report. Zimbalist was in such demand during this time that he was given a vacation by Jack L. Warner, owing to exhaustion from his busy schedule.

Jack Warner lent him to Columbia Pictures for By Love Possessed in exchange for adding several years to his Warners' contract, but he refused to let Zimbalist appear in BUtterfield 8 for Metro-Goldwyn-Mayer.[14]

In 1959, he was awarded the Golden Globe for "Most Promising Newcomer – Male".

Zimbalist in The F.B.I., first episode, 1971

Apart from 77 Sunset Strip, Zimbalist was most widely known for his starring role as Inspector Lewis Erskine in the Quinn Martin television production The F.B.I., which premiered on September 19, 1965, and aired its final episode on September 8, 1974. Zimbalist was generous in his praise of producer Martin and of his own experience starring in the show. Those who worked with him were equally admiring of the star's professionalism and likable personality.[15]

Zimbalist maintained a strong personal relationship with F.B.I. director J. Edgar Hoover, who requested that the show be technically accurate and portray his agents in the best possible light, and he insisted actors playing F.B.I. employees undergo a background check.[15] Zimbalist subsequently spent a week in contact with Hoover in Washington, D.C., and at the F.B.I. Academy in Quantico, Virginia. The men remained mutual admirers for the rest of Hoover's life.[15] Hoover held up Zimbalist as a model for F.B.I. employees' personal appearance.[16]

The Society of Former Special Agents of the Federal Bureau of Investigation[17] honored the character of Lewis Erskine in 1985 with a set of retired credentials,[18] and on June 8, 2009, FBI Director Robert Mueller presented Zimbalist with a plaque honoring him for his work on the series.[18][19]

The show was revived in the 1980s as Today's FBI starring Mike Connors.

Zimbalist in 1972

After 77 Sunset Strip, he appeared in other series, including CBS's short-lived The Reporter starring Harry Guardino as journalist Danny Taylor of the fictitious New York Globe. He also appeared in leading and supporting roles in several feature films, including Harlow, A Fever in the Blood (a film about a ruthless politician), Wait Until Dark and Airport 1975.

Zimbalist had a recurring role as Daniel Chalmers, a white-collar con man, on his daughter Stephanie Zimbalist's 1980s television detective series Remington Steele. He also recurred in the television dramatic series Hotel.

In 1990, he played the father of Zorro in the Christian Broadcasting Network's The New Zorro. Zimbalist relinquished the role after the program's first season because of the filming at studios outside Madrid, Spain, and the role subsequently went to Henry Darrow. He had a small recurring role in the 1990s hit science fiction television series Babylon 5 as William Edgars.

Also in the 1990s, Zimbalist played Alfred Pennyworth in Batman: The Animated Series as well as in Superman: The Animated Series, The New Batman Adventures, Justice League, Static Shock, and the animated films Batman: Mask of the Phantasm, Batman & Mr. Freeze: SubZero, Batman: Mystery of the Batwoman; he also played villain Doctor Octopus in Spider-Man: The Animated Series. He appeared on the Trinity Broadcasting Network[20] and as himself in the 1998 Smithsonian Institution production of Gemstones of America.[21] He performed as the narrator in "Good Morning, America" by Elinor Remick Warren.[22]

Zimbalist wrote an autobiography, My Dinner of Herbs, published by Limelight Editions, New York.[13]

In 2008, he appeared in the short film The Delivery, in which he played a professor who helps a young girl in her struggles for literacy. The film won first place in fantasy at the Dragon*Con Film Festival and was an official selection at the Los Angeles International Children's Festival and the Reel Women International Film Festival in 2009.

Zimbalist's parents, Alma Gluck and Efrem Zimbalist, were of Jewish descent but, on emigrating to America, had left the religion.[24] Moreover, Efrem Zimbalist stated, "As far as I am concerned, there has been no Jew in the family for sixty-five years."[24]

Zimbalist was baptized in the Episcopal Church. He said that when growing up he was taken to church every Sunday. He attended St. Paul's School, an Episcopal boarding school in New Hampshire.[25] Zimbalist said his faith gave him comfort when Emily died.[26]

He had a nine-year association with the practice of Transcendental Meditation as taught by Maharishi Mahesh Yogi. Zimbalist described the Maharishi Yogi as a "fascinating character", but found the meditation method "... was a total waste of energy for me."[26]

In the late 1970s, he was drawn to the Charismatic Christianity movement. His first association was with Jim Bakker and Tammy Faye Bakker's PTL ministry. For several years, he was a member of the PTL board. PTL's principal televangelistic successor, the Trinity Broadcasting Network (TBN),[27] engaged Zimbalist to make its many announcements, including the station's idents every half hour, which aired between 1992 and 2012. In a five-minute segment called "The Word" aired on TBN at 25 minutes after the hour, Zimbalist would read a verse from the Bible, eventually completing the entire text, verse by verse.[28] In 1989, he said, "for a while I did go overboard in my association with a fundamentalist group".[29]

In later life, Zimbalist joined the congregation of an Episcopal parish near to his home.[26] Afterward he joined the Anglican Church of Our Savior in Santa Barbara; he was an occasional reader there and requested donations be made to them (among others) in his obituary.[30]

In 1963 and 1964, Zimbalist joined fellow actors William Lundigan, Chill Wills and Walter Brennan in making appearances on behalf of U.S. Senator Barry Goldwater, the Republican candidate, in his election campaign against U.S. President Lyndon B. Johnson.[31]

Zimbalist died at the age of 95, the same age at which his father had died, on May 2, 2014, from natural causes.[27]